%0 Journal Article %T Towards 4-dimensional atomic force spectroscopy using the spectral inversion method %A Jeffrey C. Williams %A Santiago D. Solares %J Beilstein Journal of Nanotechnology %D 2013 %I %R 10.3762/bjnano.4.10 %X We introduce a novel and potentially powerful, yet relatively simple extension of the spectral inversion method, which offers the possibility of carrying out 4-dimensional (4D) atomic force spectroscopy. With the extended spectral inversion method it is theoretically possible to measure the tip¨Csample forces as a function of the three Cartesian coordinates in the scanning volume (x, y and z) and the vertical velocity of the tip, through a single 2-dimensional (2D) surface scan. Although signal-to-noise ratio limitations can currently prevent the accurate experimental implementation of the 4D method, and the extraction of rate-dependent material properties from the force maps is a formidable challenge, the spectral inversion method is a promising approach due to its dynamic nature, robustness, relative simplicity and previous successes. %K atomic force microscopy %K spectral inversion %K spectroscopy %K torsional harmonic cantilever %K viscoelasticity %U http://dx.doi.org/10.3762/bjnano.4.10