|
OALib Journal期刊
ISSN: 2333-9721
费用：99美元
|
|
|
|
PhotocatalyticactivityofmesoporousmicrobricksofZnOnanoparticlespreparedbythethermaldecompositionofbis(2-aminonicotinato)zinc(II)
DOI: 10.1016/S1872-2067(14)60305-3, PP. 742-749
Keywords: Znicoxide,Bis(2-aminonicotinato)zinc(II),Mesoporous,Photocatalyst,Nanoparticle
Abstract:
？Hollowmicroblocksof[Zn(anic)2],asanovelcoordinationcompound,weresynthesizedusing2-aminonicotinicacid(Hanic)andzinc(II)nitratetetrahydrate.Thechemicalcompositionofthezinccomplex,ZnC12H10N4O4,wasdeterminedbyFouriertransforminfrared(FTIR)spectroscopyandelementalanalysis.ThesynthesizedzinccomplexwasusedasaprecursortoproduceZnOnanostructuresbycalcinationat550℃for4h.MorphologicalstudiesbyscanningelectronmicroscopyandtransmissionelectronmicroscopyrevealedtheformationofporousmicrobricksofZnOnanoparticles.N2adsorption-desorptionanalysisshowedthattheobtainedZnOmicrobrickspossessamesoporousstructurewithasurfaceareaof8.13m2/gandaporesizeof22.6nm.TheX-raydiffractionpatternofthefinalproductprovedtheformationofapureZnOcompositionwithahexagonalstructure.Moreover,FTIRanalysesshowedthatthe2-aminonicotinicacidligandpeakswereabsentafterthecalcinationstep.DiffusereflectancespectroscopywasusedtodeterminethebandgapenergyoftheproducedZnOanditwasabout3.19eV.ToinvestigatethephotocatalyticactivityoftheporousZnOnanostructure,aseriesofphotocatalytictestswerecarriedouttoremoveCongored,asarepresentativetoxicazodye,fromaqueoussolution.Theresultsshowthattheproductcanbeusedasanefficientphotocatalystforwastewatertreatmentwithhighdegradationefficiency.
| [1] | Rathnayake W G I U, Ismail H, Baharin A, Bandara I M C C D, Rajapakse S. J Appl Polym Sci, 2014, 131: 39601/1
|
| [2] | Akhavan O, Azimirad R, Safa S. Mater Chem Phys, 2011, 130: 598
|
| [3] | Akhavan O, Mehrabian M, Mirabbaszadeh K, Azimirad R. J Phys D, 2009, 42: 225305/1
|
| [4] | Fang X, Wang X H, Zhao D X, Zhao H F, Fang F, Wei Z P, Li J H, Chu X Y, Wang F, Wang D D, Yan Y S. Physica E, 2014, 59: 93
|
| [5] | Nedic S, Chun Y T, Hong W K, Chu D P, Welland M. Appl Phys Lett, 2014, 104: 033101/1
|
| [6] | Chandiran A K, Abdi-Jalebi M, Nazeeruddin M K, Gr？tzel M. ACS Nano, 2014, 8: 2261
|
| [7] | Akhavan O. Carbon, 2011, 49: 11
|
| [8] | Kim M, Lee H J, Oh S, Kim Y, Jung H, Oh M K, Yoon Y J, Yoo T H, Yoon T S, Lee H H. Biosens Bioelectron, 2014, 56: 33
|
| [9] | Akhavan, O. ACS Nano, 2010, 4: 4174
|
| [10] | Zhang H, Sun J M, Dagle V L, Halevi B, Datye A K, Wang Y. ACS Catal, 2014, 4: 2379
|
| [11] | Alinezhad H, Tavakkoli S M, Biparva P. Chin J Catal (催化学报), 2014, 35: 560
|
| [12] | Lu J, Wang H H, Dong Y F, Wang F Q, Dong S J. Chin J Catal (催化学报), 2014, 35: 1113
|
| [13] | Kumar R, Anandan S, Hembram K, Narasinga Rao T. ACS Appl Mater Interf, 2014, 6: 13138
|
| [14] | Wu D Z, Fan X M, Dai J, Liu H R, Liu H, Zhang F Z. Chin J Catal (催化学报), 2012, 33: 802
|
| [15] | Wang X C, Yu J C, Ho C M, Hou Y D, Fu X Z. Langmuir, 2005, 21: 2552
|
| [16] | Chong M N, Lei S M, Jin B, Saint C, Chow C W K. Sep Purif Technol, 2009, 67: 355
|
| [17] | Xu H L, Wang W Z, Zhu W. J Phys Chem B, 2006, 110: 13829
|
| [18] | Yu J G, Su Y R, Cheng B. Adv Funct Mater, 2007, 17: 1984
|
| [19] | Soares-Santos P C R, Sá Ferreira R A, Trindade T, Carlos L D, Nogueira H I S. J Alloys Compd, 2008, 451: 575
|
| [20] | Abu-Youssef M A M, Dey R, Gohar Y, Massoud A A, ？hrstr？m L, Langer V. Inorg Chem, 2007, 46: 5893
|
| [21] | Toma M, Sanchez A, Garcia-Tasende M S, Casas J S, Castellano E E, Ellena J. Appl Organomet Chem, 2004, 18: 302
|
| [22] | Paraschiv C, Cucos A, Shova S, Madalan A M, Maxim C, Visinescu D, Cojocaru B, Parvulescu V I, Andruh M. Cryst Growth Des, 2014, DOI: 10.1021/cg501604c
|
| [23] | Kimitsuka Y, Hosono E, Ueno S, Zhou H S, Fujihara S. Inorg Chem, 2013, 52: 14028
|
| [24] | Tadjarodi A, Izadi M, Imani M. Mater Lett, 2013, 92: 108
|
| [25] | Wang X Z, Liu W, Liu J R, Wang F L, Kong J, Qiu S, He C Z, Luan L Q. ACS Appl Mater Interf, 2012, 4: 817
|
| [26] | Jamal R K, Hameed M A, Adem K A. Mater Lett, 2014, 132: 31
|
| [27] | Jin C G, Yu T, Yang Y, Wu Z F, Zhuge L J, Wu X M, Feng Z C. Mater Chem Phys, 2013, 139: 506
|
| [28] | Sakkas V A, Islam Md A, Stalikas C, Albanis T A. J Hazard Mater, 2010, 175: 33
|
| [29] | Nakamoto K. Infrared and Raman Spectra of Inorganic and Coordination Compounds. 6th Ed. New Jersey: Wiley, 2009
|
| [30] | Zhang M Y, Liu Y, Li L, Gao H, Zhang X T. Catal Commun, 2015, 58: 122
|
| [31] | Zhou M J, Gao X H, Hu Y, Chen J F, Hu X. Appl Catal B, 2013, 138-139: 1
|
| [32] | Yu J G, Xiang Q J, Zhou M H. Appl Catal B, 2009, 90: 595
|
| [33] | Sivalingam G, Nagaveni K, Hegde M S, Madras G. Appl Catal B, 2003, 45: 23
|
| [34] | Yu J G, Yu J C, Leung M K P, Ho W, Cheng B, Zhao X J, Zhao J C. J Catal, 2003, 217: 69
|
| [35] | Cao L X, Spiess F J, Huang A M, Suib S L, Obee T N, Hay S O, Freihaut J D. J Phys Chem B, 1999, 103: 2912
|
| [36] | Xiao Q, Si Z C, Zhang J, Xiao C, Tan X K. J Hazard Mater, 2008, 150: 62
|
| [37] | Huang Y, Ho W, Lee S, Zhang L Z, Li G S, Yu J C. Langmuir, 2008, 24: 3510
|
| [38] | Xiao K, Tian N, Guo Y X, Huang H W, Li X W, Zhang Y H. Inorg Chem Commun, 2015, 52: 5
|
| [39] | Comparelli R, Fanizza E, Curri M L, Cozzoli P D, Mascolo G, Agostiano A. Appl Catal B, 2005, 60: 1
|
| [40] | Zhang Y H, Chen Z, Liu S Q, Xu Y J. Appl Catal B, 2013, 140-141: 598
|
Full-Text
comments powered by
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|
