|
OALib Journal期刊
ISSN: 2333-9721
费用：99美元
|
|
|
|
原位合成具有高可见光催化活性的C3N4/CdS纳米复合材料
DOI: 10.1016/S1872-2067(14)60237-0, PP. 372-379
Keywords: 氮化碳,硫化镉,光催化,污染物降解
Abstract:
？以硫氰酸铵和氯化镉为原料,采用无模板混合高温煅烧法一步合成氮化碳/硫化镉纳米晶(C3N4/CdS)的复合半导体材料.采用X射线衍射、傅立叶变换红外光谱和透射电镜等技术对其结构和形貌进行了表征.以有机污染物罗丹明B(RhB)为模拟污染物对复合催化剂的可见光催化活性进行测试.结果表明,C3N4/CdS复合材料中CdS以六方相纳米晶的形式均匀分散;CdS的复合基本不改变C3N4主体结构及聚合度;与纯C3N4相比,复合材料在可见区的光吸收能力有所增强.合适的能带匹配有利于光生载流子的迁移,抑制了其复合速率.在可见光照射下,复合半导体能够更加快速的降解有机污染物,且保持很好的稳定性.
| [1] | Wang X C, Maeda K, Chen X F, TakaNabe K, Domen K, Hou Y D, Fu X Z, Antonietti M. J Am Chem Soc, 2009, 131: 1680
|
| [2] | Fischer A, Antonietti M, Thomas A. Adv Mater, 2007, 19: 264
|
| [3] | Kim M, Hwang S, Yu J S. J Mater Chem, 2007, 17: 1656
|
| [4] | Park S S, Chu S W, Xue C F, Zhao D Y, Ha C S. J Mater Chem, 2011, 21: 10801
|
| [5] | Lee E Z, Jun Y S, Hong W H, Thomas A, Jin M M. Angew Chem Int Ed, 2010, 49: 9706
|
| [6] | Goettmann F, Fischer A, Antonietti M, Thomas A. Angew Chem Int Ed, 2006, 45: 4467
|
| [7] | Wang Y, Wang X C, Antonietti M. Angew Chem Int Ed, 2012, 51: 68
|
| [8] | Zheng Y, Liu J, Liang J, Jaroniec M, Qiao S Z. Energy Environ Sci, 2012, 5: 6717
|
| [9] | Zhang J S, Grzelczak M, Hou Y D, Maeda K, Domen K, Fu X Z, Antonietti M, Wang X C. Chem Sci, 2012, 3: 443
|
| [10] | Cao S W, Yu J G. J Phys Chem Lett, 2014, 5: 2101
|
| [11] | Yan S C, Li Z S, Zou Z G. Langmuir, 2010, 26: 3894
|
| [12] | Lee S C, Lintang H O, Yuliati L. Chem Asian J, 2012, 7: 2139
|
| [13] | Shalom M, Inal S, Fettkenhauer C, Neher D, Antonietti M. J Am Chem Soc, 2013, 135: 7118
|
| [14] | Li X H, Antonietti M. Chem Soc Rev, 2013, 42: 6593
|
| [15] | Ye X J, Cui Y J, Wang X C. ChemSusChem, 2014, 7: 738
|
| [16] | Zhang Y J, Mori T, Ye J H, Antoniett M. J Am Chem Soc, 2010, 132: 6294
|
| [17] | Wang W J, Yu J C, Xia D H, Wong P K, Li Y C. Environ Sci Technol, 2013, 47: 8724
|
| [18] | Pan C S, Xu J, Wang Y J, Li D, Zhu Y F. Adv Funct Mater, 2012, 22: 1518
|
| [19] | Yu J G, Wang S H, Low J X, Xiao W. Phys Chem Chem Phys, 2013, 15: 16883
|
| [20] | Sun J X, Yuan Y P, Qiu L G, Jiang X, Xie A J, Shen Y H, Zhu J F. Dalton Trans, 2012, 41: 6756
|
| [21] | Fu J, Tian Y L, Chang B B, Xi F N, Dong X P. J Mater Chem, 2012, 22: 21159
|
| [22] | Zong X, Wu G P, Yan H J, Ma G J, Shi J Y, Wen F Y, Wang L, Li C. J Phys Chem C, 2010, 114: 1963
|
| [23] | Shen K, Gondal M A, Siddique R G, Shi S, Wang S Q, Sun J B, Xu Q Y. Chin J Catal (沈凯, Gondal M A, Siddique R G, 施珊, 王斯琦, 孙江波, 徐庆宇. 催化学报), 2014, 35: 78
|
| [24] | Hu Y, Gao X H, Yu L, Wang Y R, Ning J Q, Xu S J, Lou X W. Angew Chem Int Ed, 2013, 52: 5636
|
| [25] | Hirai T, Bando Y, Komasawa I. J Phys Chem B, 2002, 106: 8967
|
| [26] | Tang Z R, Yin X, Zhang Y H, Xu Y J. Inorg Chem, 2013, 52: 11758
|
| [27] | Ge L, Zuo F, Liu J K, Ma Q, Wang C, Sun D Z, Bartels L, Feng P Y. J Phys Chem C, 2012, 116: 13708
|
| [28] | Fu J, Chang B B, Tian Y L, Xi F N, Dong X P. J Mater Chem A, 2013, 1: 3083
|
| [29] | Cui Y J, Zhang J S, Zhang G G, Huang J H, Liu P, Antonietti M, Wang X C. J Mater Chem, 2011, 21: 13032
|
| [30] | Cui Y J, Huang J H, Fu X Z, Wang X C. Catal Sci Technol, 2012, 2: 1396
|
| [31] | Lotsch B V, Schnick W. Chem Mater, 2006, 18: 1891
|
| [32] | Lyth S M, Nabae Y, Moriya S, Kuroki S, Kakimoto M, Ozaki J, Miyata S. J Phys Chem C, 2009, 113: 20148
|
| [33] | Liu J, Zhang T, Wang Z, Dawson G, Chen W. J Mater Chem, 2011, 21: 14398
|
| [34] | Foy D, Demazeau G, Florian P, Massiot D, Labrugere C, Goglio G. J Solid State Chem, 2009, 182: 165
|
| [35] | Cao S W, Yuan Y P, Fang J, Shahjamali M M, Boey F Y C, Barber J, Loo S C J, Xun C. Int J Hydrogen Energy, 2013, 38, 1258
|
| [36] | Bao N Z, Shen L M, Takata T, Domen K. Chem Mater, 2008, 20: 110
|
| [37] | Jiang D W, Zhou T S, Sun Q, Yu Y Y, Shi G Y, Jin L T. Chin J Chem, 2011, 29: 2505
|
| [38] | Chen X F, Jun Y S, Takanabe K, Maeda K, Domen K, Fu X Z, Antonietti M, Wang X C. Chem Mater, 2009, 21, 4093
|
| [39] | Zhang J S, Chen X F, Takanabe K, Maeda K, Domen K, Epping J D, Fu X Z, Antonietti M, Wang X C. Angew Chem Int Ed, 2010, 49: 441
|
| [40] | Zhang J S, Zhang M W, Sun R Q, Wang X C. Angew Chem Int Ed, 2012, 51: 10145
|
| [41] | Zhang G G, Zhang M W, Ye X X, Qiu X Q, Lin S, Wang X C. Adv Mater, 2014, 26: 805
|
| [42] | Cui Y J, Ding Z X, Liu P, Antonietti M, Fu X Z, Wang X C. Phys Chem Chem Phys, 2012, 14: 1455
|
Full-Text
|
|
Contact Us
service@oalib.com QQ:3279437679 
WhatsApp +8615387084133
|
|
